Structure-Property/Activity Correlations of Coordination Compounds, Supramolecular Molecular Assemblies and Materials, with Possible Industrial and Biological Applications
DOI:
https://doi.org/10.29356/jmcs.v69i1.2317Keywords:
Coordination compounds, coordination polymers, metal-organic frameworks (MOFs), structural characterization, structure-property relationshipsAbstract
This work gives an overview of the scientific contributions developed in the research group of prof. Dr. Hiram Isaac Beltrán during the last 22 years of his career, mainly at Universidad Autónoma Metropolitana, first in Unidad Cuajimalpa and later in Unidad Azcapotzalco. During this period, research was carried out on the development of, (i) organic ligands to obtain boron-coordination compounds, (ii) diorganotin(IV) coordination compounds directly obtained by the template effect, (iii) applications and lines of research derived from the developed coordination compounds of boron and tin, (iv) coordination polymers and metal-organic frameworks (MOFs), (v) infiltrated coordination polymers and MOFs, (vi) band gap modulation and luminescence properties of coordination polymers and MOFs, (vii) biological properties of coordination polymers and MOFs, (viii) macrocyclic systems and their applications, and (ix) supramolecular assemblies and their applications. Conducting of more than 90 research papers and about 20 patents during this period. All this research involved the design and development of a specific molecular or material system with precise physicochemical properties to achieve a goal, fulfill a function or even be (multi)functional for biologic, scientific or industrial purposes. To follow all these research directions, some concepts will be highlighted in the overview and later the compendium will be presented. Acquiring this knowledge and experience has allowed us to design and develop molecular and material systems to achieve specific functions and applications. This has also helped other research groups to understand their own systems under investigation and has furthered the field of applied chemistry at a multifunctional level.
Resumen. Este trabajo ofrece una visión general de las contribuciones científicas desarrolladas en el grupo de investigación del prof. Dr. Hiram Isaac Beltrán durante los últimos 22 años de su carrera, principalmente en la Universidad Autónoma Metropolitana, primero en la Unidad Cuajimalpa y luego en la Unidad Azcapotzalco. Durante este periodo, se ha investigado el desarrollo de (i) ligandos orgánicos para la obtención de compuestos de coordinación con boro, (ii) compuestos de coordinación de diorganoestaño(IV) obtenidos directamente por efecto templado, (iii) aplicaciones y líneas de investigación derivadas de los compuestos de coordinación de boro y estaño desarrollados, (iv) polímeros de coordinación y redes metal-orgánicas (MOF), (v) infiltración de polímeros de coordinación y MOFs, (vi) modulación de banda prohibida y propiedades de luminiscencia de polímeros de coordinación y MOFs, (vii ) propiedades biológicas de polímeros de coordinación y MOFs, (viii) sistemas macrocíclicos y sus aplicaciones, y (ix) ensambles supramoleculares y sus aplicaciones.. Realizando más de 90 artículos de investigación y alrededor de 20 patentes durante este periodo. Toda esta investigación involucra el diseño y desarrollo de un sistema molecular o material particular con propiedades fisicoquímicas precisas para lograr un objetivo, para eventualmente cumplir una función o incluso ser (multi)funcional para fines biológicos, científicos o industriales. Para seguir todas estas líneas de investigación, se destacaron algunos conceptos y posteriormente se presentó el compendio. La adquisición de este conocimiento y experiencia ha permitido diseñar y desarrollar sistemas moleculares y materiales para lograr funciones y aplicaciones específicas. Esto también ha ayudado a otros grupos de investigación a comprender sus propios sistemas de estudio y ha impulsado el campo de investigación de la química aplicada a un nivel multifuncional.
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